C-H Activation by Andrew Martins, Brian Mariampillai, Mark Lautens (auth.), PDF

By Andrew Martins, Brian Mariampillai, Mark Lautens (auth.), Jin-Quan Yu, Zhangjie Shi (eds.)

ISBN-10: 3642123554

ISBN-13: 9783642123559

Table of Contents - Synthesis within the Key of Catellani: Norbornene-Mediated ortho C–H Functionalization - Mechanistic issues within the improvement and Use of Azine, Diazine and Azole N-Oxides in Palladium-Catalyzed Direct Arylation - Palladium and Copper Catalysis in Regioselective, Intermolecular Coupling of C–H and C–Hal Bonds - Pd-Catalyzed C–H Bond Functionalization at the Indole and Pyrrole Nucleus - distant C–H Activation through Through-Space Palladium and Rhodium Migrations - Palladium-Catalyzed Aryl–Aryl Bond Formation via Double C–H Activation - Palladium-Catalyzed Allylic C–H Bond Functionalization of Olefins - Ruthenium-Catalyzed Direct Arylations via C–H Bond Cleavages - Rhodium-Catalyzed C–H Bond Arylationof Arenes - Cross-Dehydrogenative Coupling Reactions of sp3-Hybridized C–H Bonds - Functionalization of Carbon–Hydrogen Bonds via Transition steel Carbenoid Insertion - Metal-Catalyzed Oxidations of C–H to C–N Bonds

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52 6 Outlook . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 53 References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 54 K. ca 36 K. 1 Biaryl Compounds in Nature and Medicinal Chemistry The biaryl structural motif is prevalent in natural products and in pharmaceutical and material sciences ([1–4]; for a review on P, N ligands with pyridyl donors see [5, 6]).

Khoury PR, Goddard JD, Tam W (2004) Tetrahedron 60:8103 14. Mizoroki T, Mori K, Ozaki A (1971) Bull Chem Soc Jpn 44:581 15. Heck RF, Nolley JP (1972) J Am Chem Soc 96:2320 16. Sicher J (1972) Angew Chem Int Ed Engl 11:200 17. Catellani M, Mealli C, Motti E, Paoli P, Perez-Carreño E, Pregosin PS (2002) J Am Chem Soc 124:4336 18. Li C-S, Jou D-C, Cheng C-H (1991) J Chem Soc Chem Commun 710 19. Catellani M, Chiusoli GP, Mari A (1984) J Organomet Chem 275:129 20. Catellani M, Chiusoli GP, Peloso C (1983) Tetrahedron Lett 24:813 21.

4 Azole N-Oxides . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 5 Methods for N-Oxide Deoxygenation . . . . . . . . . . . . . . . . . . . . . . . . . 49 4 Applications in Medicinal Chemistry . . . . . . . . . . . . . . . . . . . . . . . . . . . 51 5 Mechanistic Considerations . . . . . . . . . . . . . . . . . . . . . . . . . . . . .

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C-H Activation by Andrew Martins, Brian Mariampillai, Mark Lautens (auth.), Jin-Quan Yu, Zhangjie Shi (eds.)


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